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old filename: 1259_389251.pdf"},{"label":"Author-supplied Keywords","value":["Spectroscopy","Emission","Absorption","Lorentzian","Gaussian","Stark broadening","Doppler broadening","Electron density","Shift","Width"]},{"label":"Degree","value":["Bachelor of Arts with Departmental Honors"]},{"label":"Description","value":"

This thesis presents time-resolved optical emission spectroscopy of laser-induced plasmas generated near a water surface in an atmospheric-pressure helium environment. A pulsed Nd:YAG laser (1064 nm, 9 ns, 200 mJ) produces plasma at the focal plane and, when the water surface is positioned within a few millimeters of focus, simultaneously at the liquid surface. Spatially and spectrally resolved emission is recorded with a nanosecond-gated intensified CCD camera coupled to a 1 m spectrometer.

Two complementary temporal regimes of the He I 587.6 nm line are examined. At late times (50 ns–10 μs), the Stark-broadened Lorentzian half-width w and line-center shift d are extracted and compared with the semi-empirical impact theory of Griem (1974) and the molecular-dynamics simulations of Gigosos et al. (2014). The measured linewidths agree with both theories to within ±10% across inferred electron densities of approximately 1.5×10E17–3×10D19 cm^(-3). The dimensionless shift-to-width ratio d/w, ranging from −0.08 to −0.30, is systematically less negative than theoretical predictions but consistent with independent laboratory benchmarks at plasma temperatures of 20 000–40 000 K.

At early times (6–30 ns), a narrow Gaussian absorption dip is observed superimposed on the broad emission pedestal, attributed to resonance absorption by helium atoms in the lower excited state of the 587.6 nm transition in a cool outer layer surrounding the dense plasma core. The dip width decreases monotonically with delay, consistent with Stark broadening at outer-layer electron densities of (0.3–3)×10E17cm^(-3). The dip center is redshifted by 0.4–0.7 nm from the vacuum wavelength, in contrast to the blueshift of the late-time emission, providing a spectrally encoded signature of the density and temperature gradient between the inner and outer plasma zones. Together, these measurements develop a unified two-zone picture of the evolving helium plasma.

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