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Phase separation in polymer blends weakens the tensile strength of recycled materials, creating a barrier to effective mechanical recycling for unsorted mixed plastics. To compatibilize polymer blends, two promising strategies are dynamic crosslinks and copolymer additives. We conduct comprehensive Monte Carlo simulations of diblock copolymer additives with reactive capabilities, finding evidence of optimal additive design properties. Non-reactive additives have been studied extensively, but such a full examination for reactive additives is currently absent in the literature. For a class of short dimer additives, we find that the chemical potential for crosslinking must reach a minimum value to achieve compatibilization, with evidence of a slight monotonicity. Above the minimum chemical potential, the critical temperature for mixing drops dramatically — a result which is then shown to persist across length scales. To evaluate compatibilization for each additive design, we investigate structural order, phase behavior, and surface tension.</p>"},{"label":"Group","value":["Theses & Dissertations"]},{"label":"Digital Origin","value":["born digital"]},{"label":"Discipline","value":["Physics"]},{"label":"Date","value":"April 15, 2025"},{"label":"EDTF Date","value":"D:00 M:00 Y:2025"},{"label":"File Format","value":["application/pdf"]},{"label":"Digital Object Identifier (DOI)","value":"https://doi.org/10.14418/wes01.1.3193"},{"label":"Type","value":["Text"]}],"description":"Polymer compatibilization with applications in mixed-plastic recycling: Dynamic crosslinks and copolymer 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