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Many common material polymers (e.g. polyethylene) are derived from fossil fuels and can take hundreds or thousands of years to degrade. One method of remedying this problem is by synthesizing polymers that can be easily broken down into their monomer units under mild conditions. Ring-opening metathesis polymerization (ROMP) utilizes a ruthenium based catalyst (Grubbs 2nd and 3rd generation) to exploit the inherent ring-strain energy of cyclic species in order to open and join monomer units. The ring strain of these monomers can be manipulated through a variety of synthetic alterations to achieve the optimal energy for ROMP; instability can arise in highly strained molecules and ring opening becomes unfavorable in minimally strained monomers. Multicyclic cyclopentadiene-derivative species have been of particular interest due to the significant and controllable effects afforded by fused rings and the breadth of possible post-polymerization functionalization opportunities afforded by cyclic substituents. In particular, fused 3- and 4-member rings are being explored due to promising ring-strain energy estimates computationally obtained using Density-Functional Theory (DFT).</p>"},{"label":"Digital Identifier","value":"b2026-nielsen"},{"label":"Digital Object Identifier (DOI)","value":"https://doi.org/10.14418/a38eycbc"},{"label":"Digital Origin","value":["born digital"]},{"label":"Discipline","value":["Chemistry"]},{"label":"Date","value":"April 15, 2026"},{"label":"EDTF Date","value":"D:00 M:00 Y:2026"},{"label":"File Format","value":["application/pdf"]},{"label":"Genre","value":["theses"]},{"label":"Group","value":["Theses & Dissertations"]},{"label":"Held By","value":"Wesleyan University Library, Wesleyan University, Middletown, CT, USA"},{"label":"Language","value":["English"]},{"label":"Repository","value":["University Archives"]},{"label":"Rights","value":["In Copyright"]},{"label":"Thesis Advisor(s)","value":["Elling, 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