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author email: jluu@wesleyan.edu
old filename: 1239_379242"},{"label":"Author-supplied Keywords","value":["Gold","Characterization","Photovoltaics","Spectroscopy","Terahertz","Conductivity","Nanorod"]},{"label":"Degree","value":["Bachelor of Arts with Departmental Honors"]},{"label":"Description","value":"

Solar cell (SC) technology has been improved using a variety of novel materials, including plasmonic nanomaterials. Plasmonic materials, such as Au, Ag, and Al, are of interest due to their unique resonant interactions with certain wavelengths of light. Incorporating plasmonic nanoparticles into SCs improves the device's power conversion efficiency and performance via multiple mechanisms, including increasing light scattering within the SC and enhancing light absorption at the materials' plasmon resonance modes. However, the impact of Au nanoparticle physical properties on their conductivity properties, and how this may impact nanoparticle electronic enhancement within SCs, are not fully understood.

Despite the increasing usage of plasmonic nanomaterials in SCs for scattering and light absorption enhancement, there is a lack of literature about the electrical conductivity of the plasmonic nanoparticles, which may influence SC performance. A technique for conductivity analysis is terahertz time-domain spectroscopy (THz-TDS or TDS), which remotely probes materials for their electronic properties. It is hypothesized that nanoscale conductivity will depend on the physical properties of the nanoparticles (such as size, shape, and composition). Specifically, Au nanoparticles may follow the Drude-Smith conductivity model, due to the high number of grain boundaries limiting internanoparticle charge carrier motion.

To assess the impact of nanoparticle size, sub-100 nm Au nanorods (NRs) with low aspect ratios between 1.5 and 6.7 were synthesized. For characterization using TDS, multiple sample preparation methods were assessed, including drop casting, wet cells, and spin coating. Drop cast samples of Au NRs were assessed using TDS, providing the surprising results that Au NRs do not absorb nor conduct at THz frequencies. When present in high concentrations in a large network, Au NRs will concentrate THz frequency light, resulting in near-field enhancement. Developing the relationship between the physical and electronic properties of plasmonic nanoparticles will deepen understanding of their energy applications, improving next-generation solar cell performance.

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